高级搜索

响应面分析法优化给水污泥吸附除磷工艺

,  ,  ,  ,  ,  , 

downloadPDF

上一篇

下一篇

马宏林, 贺涛, 洪雷, 魏东洋, 李杰, 孙三祥, 许振成. 响应面分析法优化给水污泥吸附除磷工艺[J]. 环境工程学报, 2015, 9(2): 546-552. doi: 10.12030/j.cjee.20150208
引用本文: 马宏林, 贺涛, 洪雷, 魏东洋, 李杰, 孙三祥, 许振成. 响应面分析法优化给水污泥吸附除磷工艺[J]. 环境工程学报, 2015, 9(2): 546-552. doi: 10.12030/j.cjee.20150208
shu
Ma Honglin, He Tao, Hong Lei, Wei Dongyang, Li Jie, Sun Sanxiang, Xu Zhencheng. Optimization of the adsorption of phosphorus by water plant sludge using response surface methodology[J]. Chinese Journal of Environmental Engineering, 2015, 9(2): 546-552. doi: 10.12030/j.cjee.20150208
Citation: Ma Honglin, He Tao, Hong Lei, Wei Dongyang, Li Jie, Sun Sanxiang, Xu Zhencheng. Optimization of the adsorption of phosphorus by water plant sludge using response surface methodology[J]. Chinese Journal of Environmental Engineering, 2015, 9(2): 546-552. doi: 10.12030/j.cjee.20150208
shu

响应面分析法优化给水污泥吸附除磷工艺

  • 1.

    兰州交通大学环境与市政工程学院, 兰州 730070

  • 2.

    环境保护部华南环境科学研究所, 广州 510655

  • 基金项目:

    国家"水体污染控制与治理"科技重大专项(2012ZX07206-004-002)

    中央级公益性科研项目(PM-zx021-201211-128 )

  • 中图分类号: X703.1

Optimization of the adsorption of phosphorus by water plant sludge using response surface methodology

  • 1.

    School of Environmental and Municipal Engineering, Lanzhou Jiaotong University, Lanzhou 730070, China

  • 2.

    South China Institute of Environmental Sciences, Ministry of Environmental Protection, Guangzhou 510655, China

  • Fund Project:

  • 摘要: 以给水污泥为吸附材料,对模拟含磷废水进行了吸附研究。在单因素实验基础上,选取投加量、pH和粒径3种因素为影响因子,以磷的去除率为响应值,采用Box-Behnken响应面分析法(BBD)研究了3种因素对磷去除率的影响以及各因素间的交互作用。建立了二次多项式回归方程预测模型,成功预测出最佳除磷工艺条件为污泥投加量3.88 g/L,pH=3.00,粒径1.00 mm,该条件下磷的去除率可达95.13%.因此,响应面分析法是优化给水污泥吸附除磷工艺的可行方法。
    Abstract: The water plant sludge was used to investigate the adsorption of phosphorus in simulated phosphorus containing wastewater as the absorbent. Based on the single factor experiment, using Box-Behnken design matrix in response surface methodology, dosage, pH and particle size were perfectly employed to study interactive effects of different factors and optimization of phosphorus removal. A predictive model of quadratic polynomial regression equation as well as optimum level values were founded successfully. The optimum conditions of phosphorus removal were determined to be dosage of 3.88 g/L,pH=3.00,particle size of 1.00 mm, the removal rate of phosphorus was up to 95.13% under the optimal conditions.Thus the response surface methodology could be viable to optimize the process of removing phosphorus.
  • 加载中
  • [1] Makris K. C., El-Shall H., Harris W. G., et al. Intraparticle phosphorus diffusion in a drinking water treatment residual at room temperature. Journal of Colloid and Interface Science, 2004, 277(2): 417-423
    [2] 袁东海, 景丽洁, 张孟群, 等. 几种人工湿地基质净化磷素的机理. 中国环境科学, 2004, 24(5): 614-617 Yuan Donghai, Jing Lijie, Zhang Mengqun, et al. Mechanism of phosphorus purification in some kinds of substrates constructed wetland systems. China Environmental Science, 2004, 24(5): 614-617 (in Chinese)
    [3] Yang Y., Tomlinson D., Kennedy S., et al. Dewatered alum sludge:A potential adsorbent for phosphorus removal. Water Science and Technology, 2006, 54(5): 207-213
    [4] 胡文华, 吴慧芳, 徐明, 等. 聚合氯化铝污泥对磷的吸附动力学及热力学. 环境工程学报, 2011, 5(10): 2287-2292 Hu Wenhua, Wu Huifang, Xu Ming, et al. Study on kinetics and thermodynamics of phosphorus adsorption onto PAC sludge. Chinese Journal of Environmental Engineering, 2011, 5(10): 2287-2292 (in Chinese)
    [5] 王昌辉, 裴元生. 给水处理厂废弃铁铝泥对正磷酸盐的吸附特征. 环境科学, 2011, 32(8): 2371-2377 Wang Changhui, Pei Yuansheng. Characteristics of orthophosphate adsorption on ferric-alum residuals (FARs) from drinking water treatment plant. Environmental Science, 2011, 32(8): 2371-2377 (in Chinese)
    [6] Sotero-Santos R. B., Rocha O., Povinelli J. Evaluation of water treatment sludges toxicity using the Daphnia bioassay. Water Research, 2005, 39(16): 3909-3917
    [7] Gibbons M. K., Gagnon G. A. Adsorption of arsenic from a Nova Scotia groundwater onto water treatment residual solids. Water Research, 2010, 44(19): 5740-5749
    [8] 林璐, 胥嘉瑞, 吴昊, 等. 不同粒径铁铝泥对砷(Ⅲ)的吸附效果. 环境科学, 2013, 34(7): 2758-2765 Lin Lu, Xu Jiarui, Wu Hao, et al. Effectiveness of arsenite adsorption by ferric and alum water treatment residuals with different grain sizes. Environmental Science, 2013, 34(7): 2758-2765 (in Chinese)
    [9] 刘超, 杨永哲, 宛娜. 铝污泥吸附六价铬的特征和机理. 环境工程学报, 2013, 7(1): 97-102 Liu Chao, Yang Yongzhe, Wan Na. Characteristic and mechanisms of chromium(Ⅵ) adsorption on alum sludge. Chinese Journal of Environmental Engineering, 2013, 7(1): 97-102 (in Chinese)
    [10] 郑怀礼, 焦世珺, 邓晓莉, 等. 响应面法优化聚磷硫酸铁的制备及其应用. 环境工程学报, 2012, 6(1): 9-14 Zheng Huaili, Jiao Shijun, Deng Xiaoli, et al. Optimization of preparation and application of PPFS by response surface methodology. Chinese Journal of Environmental Engineering, 2012, 6(1): 9-14 (in Chinese)
    [11] Sadri Moghaddam S., Alavi Moghaddam M. R., Arami M. Coagulation/flocculation process for dye removal using sludge from water treatment plant: optimization through response surface methodology. Journal of Hazardous Materials, 2010, 175(1): 651-657
    [12] 陈颖, 杨朝晖, 李小江, 等. 茶树菇废菌体对水中Cr (Ⅵ) 吸附的响应面优化及机理研究. 环境科学学报, 2010, 30(8): 1593-1600 Chen Ying, Yang Zhaohui, Li Xiaojiang, et al.Biosorption of Cr(Ⅵ) from aqueous solutions by waste Agrocybe aegerita: Optimization and mechanism. Acta Scientiae Circumstantiae, 2010, 30(8): 1593-1600(in Chinese)
    [13] 陈毅忠, 王利平, 杜尔登, 等. 自来水厂脱水铝污泥对水中磷的吸附去除研究. 中国给水排水, 2011, 27(23): 88-91 Chen Yizhong, Wang Liping, Du Erdeng, et al. Adsorption removal of phosphorus from wastewater by dewatered alum sludge from waterworks. China Water & Wastewater, 2011, 27(23): 88-91 (in Chinese)
    [14] Irawan C., Liu J. C., Wu C. C. Removal of boron using aluminum-based water treatment residuals (Al-WTRs). Desalination, 2011, 276(1): 322-327
    [15] Yang Y., Zhao Y. Q. Babatunde A. O., et al. Characteristics and mechanisms of phosphate adsorption on dewatered alum sludge. Separation and Purification Technology, 2006, 51(2): 193-200
    [16] 李璐, 杨朝晖, 孙珮石, 等. 基于响应面优化条件下柚皮对Pb2+的吸附. 环境科学学报, 2009, 29(7): 1426-1433 Li L.u, Yang Zhaohui, Sun Peishi, et al. Optimization of the biosorption of Pb2+ by citron peel using response surface methodology. Acta Scientiae Circumstantiae, 2009, 29(7): 1426-1433 (in Chinese)
    [17] Babatunde A. O., Zhao Y. Q., Burke A. M., et al. Characterization of aluminium-based water treatment residual for potential phosphorus removal in engineered wetlands. Environmental Pollution, 2009, 157(10): 2830-2836
    [18] Chakravarty S., Mohanty A., Sudha T. N., et al. Removal of Pb(II) ions from aqueous solution by adsorption using bael leaves (Aegle marmelos). Journal of Hazardous Materials, 2010, 173(1-3): 502-509
    [19] 赵雪松, 胡小贞, 卢少勇, 等. 不同粒径方解石在不同pH值时对磷的等温吸附特征与吸附效果. 环境科学学报, 2008, 28(9): 1872-1877 Zhao Xuesong, Hu Xiaozhen, Lu Shaoyong, et al. Phosphorus sorption by natural calcite and the effects of pH and grain size. Acta Scientiae Circumstantiae, 2008, 28(9): 1872-1877(in Chinese)
    [20] 梁小燕, 程建华, 胡勇有, 等. VUV/Fe3+体系对水中全氟辛酸(PFOA)脱氟影响因素研究. 环境科学学报, 2013, 33(9): 2432-2438 Liang Xiaoyan, Cheng Jianhua, Hu Yongyou, et al. The influencing factors on defluorination of aqueous perfluorooctanoic acid (PFOA) by VUV/Fe3+ system. Acta Scientiae Circumstantiae, 2013, 33(9): 2432-2438(in Chinese)
    [21] Sadri Moghaddam S., Alavi Moghaddam M. R., Arami M. Coagulation/flocculation process for dye removal using sludge from water treatment plant: Optimization through response surface methodology. Journal of Hazardous Materials, 2010, 175(1-3): 651-657
    [22] Wang Jianping, Chen Yongzhen, Wang Yi, et al. Optimization of the coagulation-flocculation process for pulp mill wastewater treatment using a combination of uniform design and response surface methodology. Water Research, 2011, 45(17): 5633-5640
    [23] Jung K. W., Kim D. H., Kim H. W., et al. Optimization of combined (acid + thermal) pretreatment for fermentative hydrogen production from Laminaria japonica using response surface methodology (RSM). International Journal of Hydrogen Energy, 2011, 36(16): 9626-9631
    [24] 魏健, 宋永会, 赵乐, 等. 响应面法优化Fenton预处理干法腈纶废水. 环境工程学报, 2013, 7(5): 1695-1701 Wei Jian, Song Yonghui, Zhao Le, et al. Optimization of Fenton process for pretreatment of dry-spun acrylic fiber wastewater with response surface methodology. Chinese Journal of Environmental Engineering, 2013, 7(5): 1695-1701 (in Chinese)
  • 加载中
WeChat 点击查看大图
计量
  • 文章访问数:  2696
  • HTML全文浏览数:  1986
  • PDF下载数:  825
  • 施引文献:  0
出版历程
  • 收稿日期:  2014-10-21
  • 刊出日期:  2015-02-07
马宏林, 贺涛, 洪雷, 魏东洋, 李杰, 孙三祥, 许振成. 响应面分析法优化给水污泥吸附除磷工艺[J]. 环境工程学报, 2015, 9(2): 546-552. doi: 10.12030/j.cjee.20150208
引用本文: 马宏林, 贺涛, 洪雷, 魏东洋, 李杰, 孙三祥, 许振成. 响应面分析法优化给水污泥吸附除磷工艺[J]. 环境工程学报, 2015, 9(2): 546-552. doi: 10.12030/j.cjee.20150208
shu
Ma Honglin, He Tao, Hong Lei, Wei Dongyang, Li Jie, Sun Sanxiang, Xu Zhencheng. Optimization of the adsorption of phosphorus by water plant sludge using response surface methodology[J]. Chinese Journal of Environmental Engineering, 2015, 9(2): 546-552. doi: 10.12030/j.cjee.20150208
Citation: Ma Honglin, He Tao, Hong Lei, Wei Dongyang, Li Jie, Sun Sanxiang, Xu Zhencheng. Optimization of the adsorption of phosphorus by water plant sludge using response surface methodology[J]. Chinese Journal of Environmental Engineering, 2015, 9(2): 546-552. doi: 10.12030/j.cjee.20150208
shu

响应面分析法优化给水污泥吸附除磷工艺

  • 1.  兰州交通大学环境与市政工程学院, 兰州 730070
  • 2.  环境保护部华南环境科学研究所, 广州 510655
  • 收稿日期:  2014-10-21
基金项目:

国家"水体污染控制与治理"科技重大专项(2012ZX07206-004-002)

中央级公益性科研项目(PM-zx021-201211-128 )

摘要: 以给水污泥为吸附材料,对模拟含磷废水进行了吸附研究。在单因素实验基础上,选取投加量、pH和粒径3种因素为影响因子,以磷的去除率为响应值,采用Box-Behnken响应面分析法(BBD)研究了3种因素对磷去除率的影响以及各因素间的交互作用。建立了二次多项式回归方程预测模型,成功预测出最佳除磷工艺条件为污泥投加量3.88 g/L,pH=3.00,粒径1.00 mm,该条件下磷的去除率可达95.13%.因此,响应面分析法是优化给水污泥吸附除磷工艺的可行方法。

English Abstract

    全文HTML

参考文献 (24)

返回顶部

目录

/

返回文章
返回

Copyright © 2019 中国科学院生态环境研究中心