北运河沉积物/水界面上重金属迁移转化规律

杨振东, 聂玉伦, 胡春. 北运河沉积物/水界面上重金属迁移转化规律[J]. 环境工程学报, 2012, 6(10): 3455-3459.
引用本文: 杨振东, 聂玉伦, 胡春. 北运河沉积物/水界面上重金属迁移转化规律[J]. 环境工程学报, 2012, 6(10): 3455-3459.
Yang Zhendong, Nie Yulun, Hu Chun. Migration and transformation of heavy metals at solid/water interface in Beiyunhe River[J]. Chinese Journal of Environmental Engineering, 2012, 6(10): 3455-3459.
Citation: Yang Zhendong, Nie Yulun, Hu Chun. Migration and transformation of heavy metals at solid/water interface in Beiyunhe River[J]. Chinese Journal of Environmental Engineering, 2012, 6(10): 3455-3459.

北运河沉积物/水界面上重金属迁移转化规律

  • 基金项目:

    国家"十一五"水专项(2008ZX07209-001)

  • 中图分类号: X53

Migration and transformation of heavy metals at solid/water interface in Beiyunhe River

  • Fund Project:
  • 摘要: 分析测定了6种元素(Cr、Co、Mn、Cu、Pb、Zn)在北运河水系10个采样点水体和表层沉积物中的含量和形态分布,利用SPSS 19.0统计软件对重金属在不同形态中的含量进行相关性分析。结果显示,北运河下游重金属污染程度高于上游;Cr、Cu、Pb、Zn在底泥可提取态中所占比例相当高,多数采样点都超过10.0%。所研究的重金属多数在底泥Fe-Mn结合态与悬浮物、可交换态、硫化物和有机质结合态均存在相关性;Mn是北运河地化循环中最为活跃的元素。
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  • [1] 郝立波,孙立吉,陆继龙,等.第二松花江中上游悬浮物重金属元素分布特征.吉林大学学报(地球科学版),2010,40(2):327-361 Hao L.B.,Sun L.J.,Lu Jilong,et al.Distribution characteristics of the heavy metals of the suspended solids in the upper and middle reaches of the Second Songhua River.Journal of Jilin University(Earth Science Edition),2010,40(2):327-361(in Chinese)
    [2] Yuan C.G.,Shi J.B.,He B.,et al.Speciation of heavy metals in marine sediments from the East China Sea by ICP-MS with sequential extraction.Environment International,2004,30(6):769-783
    [3] Dragovic S.,Mihailovic N.,Gajic B.Heavy metals in soils:Distribution,relationship with soil characteristics and radionuclides and multivariate assessment of contamination sources.Chemosphere,2008,72(3):491-495
    [4] 郑毅.北运河流域洪水预报与调度系统研究及应用.北京:清华大学博士学位论文,2009 Zheng Y.Flood risk management decision support systems of the Beiyunhe River basin.Beijing:Doctoral Dissertation of Tsinghua University,2009(in Chinese)
    [5] 何太蓉,刘存东,庄红娟.重庆市清水溪河流沉积物重金属污染及潜在生态风险评价.环境工程学报,2009,3(7):1329-1332 He T.R.,Liu C.D.,Zhuang H.J.Pollution of heavymetals in the sediments from Qingshui Stream in Chongqing and its potential ecological risk assessment.Chinese Journal of Environmental Engineering,2009,3(7):1329-1332(in Chinese)
    [6] Tessier A.,Campbell P.G.C.,Blsson M.Sequential extraction procedure for the speciation of particulate trace metals.Analytical Chemistry,1979,51(7):844-850
    [7] 赵锁志,刘丽萍,王喜宽,等.黄河内蒙古段上覆水、悬浮物和底泥重金属特征及生态风险研究.现代地质,2008,22(2):304-312 Zhao S.Z.,Liu L.P.,Wang X.K.,et al.Characteristics and ecological risk of heavy metals in overlying water,suspended particles and bed mud in the Inner Mongolia Stretch of the Yellow River.Geoscience,2008,22(2):304-312 (in Chinese)
    [8] Yuan C.,Jiang G.,Liang L.,et al.Sequential extraction of some heavy metals in Haihe River sediments,People's Republic of China.Bulletin Environmental Contamination and Toxicology,2004,73(1):59-66
    [9] Meng Y.T.,Zheng Y.M.,Zhang L.W.,et al.Biogenic Mn oxides for effective adsorption of Cd from aquatic environment.Environmental Pollution,2009,157(8):2577-2583
    [10] Taillefert M.,Macgregor B.J.,Gailard J.F.,et al.Evidence for a dynamic cycle between Mn and Co in the water column of a stratified lake.Environmental Science & Technology,2002,36(3):468-476
    [11] Konstantinos C.C.,Sun U.,Yiannis D.Effect of metal ions on the indigenous radicals of humic acids:High field electron paramagnetic resonance study.Environmental Science & Technology,2010,44(18):7011-7016
    [12] Tokalio S.,Kartal S.,Elci L.Determination of heavy metals and their speciation in lake sediments by flame atomic absorption spectrometry after a four-stage sequential extraction procedure.Analytica Chimica Acta,2000,413(1):33-40
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出版历程
  • 收稿日期:  2011-09-05
  • 刊出日期:  2012-10-16
杨振东, 聂玉伦, 胡春. 北运河沉积物/水界面上重金属迁移转化规律[J]. 环境工程学报, 2012, 6(10): 3455-3459.
引用本文: 杨振东, 聂玉伦, 胡春. 北运河沉积物/水界面上重金属迁移转化规律[J]. 环境工程学报, 2012, 6(10): 3455-3459.
Yang Zhendong, Nie Yulun, Hu Chun. Migration and transformation of heavy metals at solid/water interface in Beiyunhe River[J]. Chinese Journal of Environmental Engineering, 2012, 6(10): 3455-3459.
Citation: Yang Zhendong, Nie Yulun, Hu Chun. Migration and transformation of heavy metals at solid/water interface in Beiyunhe River[J]. Chinese Journal of Environmental Engineering, 2012, 6(10): 3455-3459.

北运河沉积物/水界面上重金属迁移转化规律

  • 1. 中国科学院生态环境研究中心环境水质学国家重点实验室, 北京 100085
基金项目:

国家"十一五"水专项(2008ZX07209-001)

摘要: 分析测定了6种元素(Cr、Co、Mn、Cu、Pb、Zn)在北运河水系10个采样点水体和表层沉积物中的含量和形态分布,利用SPSS 19.0统计软件对重金属在不同形态中的含量进行相关性分析。结果显示,北运河下游重金属污染程度高于上游;Cr、Cu、Pb、Zn在底泥可提取态中所占比例相当高,多数采样点都超过10.0%。所研究的重金属多数在底泥Fe-Mn结合态与悬浮物、可交换态、硫化物和有机质结合态均存在相关性;Mn是北运河地化循环中最为活跃的元素。

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