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膜接触法捕集生物质气CO2的研究进展

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鹿莎莎, 黄川, 申亚栋, 葛春玲, 王里奥. 膜接触法捕集生物质气CO2的研究进展[J]. 环境化学, 2021, (4): 1088-1099. doi: 10.7524/j.issn.0254-6108.2020082404
引用本文: 鹿莎莎, 黄川, 申亚栋, 葛春玲, 王里奥. 膜接触法捕集生物质气CO2的研究进展[J]. 环境化学, 2021, (4): 1088-1099. doi: 10.7524/j.issn.0254-6108.2020082404
shu
LU Shasha, HUANG Chuan, SHEN Yadong, GE Chunling, WANG Li. Research progress of membrane contactor technology on CO2 Capture[J]. Environmental Chemistry, 2021, (4): 1088-1099. doi: 10.7524/j.issn.0254-6108.2020082404
Citation: LU Shasha, HUANG Chuan, SHEN Yadong, GE Chunling, WANG Li. Research progress of membrane contactor technology on CO2 Capture[J]. Environmental Chemistry, 2021, (4): 1088-1099. doi: 10.7524/j.issn.0254-6108.2020082404
shu

膜接触法捕集生物质气CO2的研究进展

  • 1. 重庆大学煤矿灾害动力学与控制国家重点实验室, 重庆, 400044;

  • 2. 重庆大学环境与生态学院, 重庆, 400045;

  • 3. 北京城市矿产资源开发有限公司, 北京, 100101

    • 通讯作者: 黄川, E-mail: hclsjb@163.com ; 
  • 基金项目:

    国家重点研发计划（2019YFC1906100），重庆市研究生科研创新项目（CYS18018）和中央高校配套资金（2020CDCGHJ014）资助.

Research progress of membrane contactor technology on CO2 Capture

  • 1. State Key Laboratory of Coal Mine Disaster Dynamics and Control, Chongqing University, Chongqing, 400044, China;

  • 2. College of Environment and Ecology, Chongqing University, Chongqing, 400045, China;

  • 3. Beijing City Mineral Resources Development Co. LTD, Beijing, 100101, China

    • Corresponding author: HUANG Chuan, hclsjb@163.com ; 
  • Fund Project: Supported by:National Key Research and Development Program of China(2019YFC1906100), Chongqing Postgraduate Scientific Research and Innovation Project(CYS18018) and the Fundamental Research Funds for the Central Universities (2020CDCGHJ014).

  • 摘要: 生物质气中CO2捕集及CH4的回收利用具有巨大经济价值和环境效益，受到各领域的广泛关注.基于中空纤维膜的气-液膜接触技术以其效率高、能耗少和操作灵活等优势被认为是CO2捕集领域的重大突破.本文以中空纤维膜材料为中心，回顾了近十年来无机膜、传统有机聚合膜、有机微孔聚合膜、混合基质膜和固定载体膜的研究和发展，论述了各类中空纤维膜的CO2捕集性能以及当前面临的挑战.同时从膜润湿、吸收剂以及工艺条件等方面分析了影响CO2分离性能的主要因素.并提出开发低成本、高CO2捕集性能和高稳定性的新型中空纤维膜以及推进膜的中试和示范试点工程作为未来发展的主流方向.
    Abstract: CO2 capture and CH4 recovery from biomass gas have great economic value and environmental benefit, and they have been widely concerned in various fields. Gas-liquid membrane contactor technology based on hollow fiber membrane is considered a major breakthrough in the field of CO2 capture due to its high separation efficiency, low energy consumption and flexible operation. Focusing on hollow fiber membrane materials, this paper reviewed detailly about the research and development of inorganic membranes, organic polymer membranes, mixed matrix membranes, and fixed-site-carrier membranes in the past decade, and introduced the gas separation performance and current challenges of various hollow fiber membranes, respectively. At the same time, the main factors (membrane wetting, absorbent and operation conditions) affecting CO2 separation performance of the hollow fiber membrane contactor were analyzed. This paper proposes that future research should focus on creating new hollow fiber membranes with low-cost, high performance of CO2 separation, high stability and the development of the membranes with excellent performance for pilot test.
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  • 收稿日期:  2020-08-24
鹿莎莎, 黄川, 申亚栋, 葛春玲, 王里奥. 膜接触法捕集生物质气CO2的研究进展[J]. 环境化学, 2021, (4): 1088-1099. doi: 10.7524/j.issn.0254-6108.2020082404
引用本文: 鹿莎莎, 黄川, 申亚栋, 葛春玲, 王里奥. 膜接触法捕集生物质气CO2的研究进展[J]. 环境化学, 2021, (4): 1088-1099. doi: 10.7524/j.issn.0254-6108.2020082404
shu
LU Shasha, HUANG Chuan, SHEN Yadong, GE Chunling, WANG Li. Research progress of membrane contactor technology on CO2 Capture[J]. Environmental Chemistry, 2021, (4): 1088-1099. doi: 10.7524/j.issn.0254-6108.2020082404
Citation: LU Shasha, HUANG Chuan, SHEN Yadong, GE Chunling, WANG Li. Research progress of membrane contactor technology on CO2 Capture[J]. Environmental Chemistry, 2021, (4): 1088-1099. doi: 10.7524/j.issn.0254-6108.2020082404
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膜接触法捕集生物质气CO2的研究进展

    通讯作者: 黄川, E-mail: hclsjb@163.com ; 
  • 1. 重庆大学煤矿灾害动力学与控制国家重点实验室, 重庆, 400044;
  • 2. 重庆大学环境与生态学院, 重庆, 400045;
  • 3. 北京城市矿产资源开发有限公司, 北京, 100101
  • 收稿日期:  2020-08-24
基金项目:

国家重点研发计划（2019YFC1906100），重庆市研究生科研创新项目（CYS18018）和中央高校配套资金（2020CDCGHJ014）资助.

摘要: 生物质气中CO2捕集及CH4的回收利用具有巨大经济价值和环境效益，受到各领域的广泛关注.基于中空纤维膜的气-液膜接触技术以其效率高、能耗少和操作灵活等优势被认为是CO2捕集领域的重大突破.本文以中空纤维膜材料为中心，回顾了近十年来无机膜、传统有机聚合膜、有机微孔聚合膜、混合基质膜和固定载体膜的研究和发展，论述了各类中空纤维膜的CO2捕集性能以及当前面临的挑战.同时从膜润湿、吸收剂以及工艺条件等方面分析了影响CO2分离性能的主要因素.并提出开发低成本、高CO2捕集性能和高稳定性的新型中空纤维膜以及推进膜的中试和示范试点工程作为未来发展的主流方向.

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