用数值模拟方法研究含硫颗粒物生成过程

郭兴明, 邢亚平. 用数值模拟方法研究含硫颗粒物生成过程[J]. 环境工程学报, 2016, 10(4): 1869-1873. doi: 10.12030/j.cjee.20160446
引用本文: 郭兴明, 邢亚平. 用数值模拟方法研究含硫颗粒物生成过程[J]. 环境工程学报, 2016, 10(4): 1869-1873. doi: 10.12030/j.cjee.20160446
Guo Xingming, Xing Yaping. Investigation of sulfur-containing particles generation by numerical simulation[J]. Chinese Journal of Environmental Engineering, 2016, 10(4): 1869-1873. doi: 10.12030/j.cjee.20160446
Citation: Guo Xingming, Xing Yaping. Investigation of sulfur-containing particles generation by numerical simulation[J]. Chinese Journal of Environmental Engineering, 2016, 10(4): 1869-1873. doi: 10.12030/j.cjee.20160446

用数值模拟方法研究含硫颗粒物生成过程

  • 基金项目:

    国家自然科学基金资助项目(20807005)

  • 中图分类号: X513

Investigation of sulfur-containing particles generation by numerical simulation

  • Fund Project:
  • 摘要: 为了研究不同燃烧条件对燃煤中含硫颗粒物生成的影响,利用数值分析方法模拟炉膛煤燃烧。通过改变燃烧环境温度、进口氧气所占总气体摩尔比,分析得到的碳烟(soot)颗粒、SO2和CO2等主要物质浓度场。模拟结果能够很好地反映炉膛内各物质生成趋势和历程。生成的碳烟颗粒中富集煤中一部分硫元素,燃烧后期未被氧化的碳烟颗粒是燃煤烟气含硫颗粒物的一个重要来源。进口O2摩尔比从0.1~0.5时碳烟颗粒迅速被氧化,出口处产生含硫碳烟颗粒物减少。在1 200~1 600 K范围内,温度增高不利于碳烟颗粒的生成,来源于碳烟颗粒的含硫颗粒物也就逐渐减少。
  • 加载中
  • [1] 赵成美,孙俊民,邓寅生,等.燃煤飞灰中细颗粒物(PM2.5)的物理化学特性.环境科学研究,2004,17(2):71-73 Zhao Chengmei,Sun Junmin,Deng Yinsheng,et al.Physiochemical characteristic of fine particle (PM2.5) in fly ash from coal combustion.Research of Environmental Science,2004,17(2):71-73(in Chinese)
    [2] 毛建雄,毛健全,赵树民.煤的清洁燃烧.北京:科学出版社,1998:5-6
    [3] 杨林军.燃烧源细颗粒物污染控制技术.北京:化学工业出版社,2011:6-9
    [4] 熊刚.煤和生物质燃烧碳烟生成的实验研究.北京:清华大学博士学位论文,2011 Xiong Gang.Experimental study of soot formation during the combustion of coal and biomass.Beijing:Doctor Dissertation of Tsinghua University,2011(in Chinese)
    [5] Turns S.R.An Introduction to Combustion:Concepts and Applications (2nd ed).Singapore:McGraw-Hill,2000:222-232
    [6] Glassman I.Sooting laminar diffusion flames:Effect of dilution,additives,pressure,and microgravity.Symposium (International) on Combustion,1998,27(1):1589-1596
    [7] Glassman I.Soot formation in combustion processes.Symposium (International) on Combustion,1989,22(1):295-311
    [8] 岑可法,姚强,骆仲泱,等.高等燃烧学.杭州:浙江大学出版社,2002:264-271
    [9] Bockhorn H.Soot Formation in Combustion.Mechanisms and models,Berlin:Springer,1994:3-19
    [10] Richter H.,Howard J.B.Formation of polycyclic aromatic hydrocarbons and their growth to soot:A review of chemical reaction pathways.Progress in Energy and Combustion Science,2000,26(4-6):565-608
    [11] Sui Jiancai,Xu Minghou,Qiu Jihua,et al.Numerical simulation of ash vaporization during pulverized coal combustion in the laboratory-scale single-burner furnace.Energy & Fuels,2005,19(4):1536-1541
    [12] Frenklach M.Reaction mechanism of soot formation in flames.Physical Chemistry Chemical Physics,2002,4(11):2028-2037
    [13] Fitzpatrick E.M.,Jones J.M.,Pourkashanian M.,et al.Mechanistic aspects of soot formation from the combustion of pine wood.Energy & Fuels,2008,22(6):3771-3778
    [14] Fitzpatrick E.M.,Bartle K.D.,Kubacki M.L.,et al.The mechanism of the formation of soot and other pollutants during the co-firing of coal and pine wood in a fixed bed combustor.Fuel,2009,88(12):2409-2417
    [15] 周浩生,陆继东.流化床内煤粒燃烧过程的数值模拟.中国电机工程学报,2004,24(12):212-217 Zhou Haosheng,Lu Jidong.Coal combustion in a fluidized bed with DEM-LES simulation.Proceedings of the CSEE,2004,24(12):212-217(in Chinese)
  • 加载中
计量
  • 文章访问数:  2010
  • HTML全文浏览数:  1559
  • PDF下载数:  875
  • 施引文献:  0
出版历程
  • 收稿日期:  2014-12-26
  • 刊出日期:  2016-04-15
郭兴明, 邢亚平. 用数值模拟方法研究含硫颗粒物生成过程[J]. 环境工程学报, 2016, 10(4): 1869-1873. doi: 10.12030/j.cjee.20160446
引用本文: 郭兴明, 邢亚平. 用数值模拟方法研究含硫颗粒物生成过程[J]. 环境工程学报, 2016, 10(4): 1869-1873. doi: 10.12030/j.cjee.20160446
Guo Xingming, Xing Yaping. Investigation of sulfur-containing particles generation by numerical simulation[J]. Chinese Journal of Environmental Engineering, 2016, 10(4): 1869-1873. doi: 10.12030/j.cjee.20160446
Citation: Guo Xingming, Xing Yaping. Investigation of sulfur-containing particles generation by numerical simulation[J]. Chinese Journal of Environmental Engineering, 2016, 10(4): 1869-1873. doi: 10.12030/j.cjee.20160446

用数值模拟方法研究含硫颗粒物生成过程

  • 1. 北京理工大学材料学院, 北京市环境科学与工程重点实验室, 北京 100081
基金项目:

国家自然科学基金资助项目(20807005)

摘要: 为了研究不同燃烧条件对燃煤中含硫颗粒物生成的影响,利用数值分析方法模拟炉膛煤燃烧。通过改变燃烧环境温度、进口氧气所占总气体摩尔比,分析得到的碳烟(soot)颗粒、SO2和CO2等主要物质浓度场。模拟结果能够很好地反映炉膛内各物质生成趋势和历程。生成的碳烟颗粒中富集煤中一部分硫元素,燃烧后期未被氧化的碳烟颗粒是燃煤烟气含硫颗粒物的一个重要来源。进口O2摩尔比从0.1~0.5时碳烟颗粒迅速被氧化,出口处产生含硫碳烟颗粒物减少。在1 200~1 600 K范围内,温度增高不利于碳烟颗粒的生成,来源于碳烟颗粒的含硫颗粒物也就逐渐减少。

English Abstract

参考文献 (15)

返回顶部

目录

/

返回文章
返回