硫酸铵作为人工气溶胶模拟尘源的研究

邓高峰; 李增和; 胡露露; 王智超; 郜津慧

doi:10.12030/j.cjee.201509193

环境工程学报

硫酸铵作为人工气溶胶模拟尘源的研究

, , , ,

邓高峰, 李增和, 胡露露, 王智超, 郜津慧. 硫酸铵作为人工气溶胶模拟尘源的研究[J]. 环境工程学报, 2017, 11(2): 977-982. doi: 10.12030/j.cjee.201509193

引用本文:

邓高峰, 李增和, 胡露露, 王智超, 郜津慧. 硫酸铵作为人工气溶胶模拟尘源的研究[J]. 环境工程学报, 2017, 11(2): 977-982. doi: 10.12030/j.cjee.201509193

DENG Gaofeng, LI Zenghe, HU Lulu, WANG Zhichao, GAO Jinhui. Research on ammonium sulfate as artificial aerosol simulated dust source[J]. Chinese Journal of Environmental Engineering, 2017, 11(2): 977-982. doi: 10.12030/j.cjee.201509193

Citation:

DENG Gaofeng, LI Zenghe, HU Lulu, WANG Zhichao, GAO Jinhui. Research on ammonium sulfate as artificial aerosol simulated dust source[J]. Chinese Journal of Environmental Engineering, 2017, 11(2): 977-982. doi: 10.12030/j.cjee.201509193

硫酸铵作为人工气溶胶模拟尘源的研究

1.
北京化工大学理学院, 北京 100029
2.
中国建筑科学研究院建筑环境与安全国家重点实验室, 北京 100013
3.
建研科技股份有限公司, 北京 100013
基金项目:
国家科技支撑计划项目（2013BAK12B03）

Research on ammonium sulfate as artificial aerosol simulated dust source

1.
College of Science, Beijing University of Chemical Technology, Beijing 100029, China
2.
State Key Laboratory of Building Safety and Built Environment, China Academy of Building Research, Beijing 100013, China
3.
Cabr Technology Co. Ltd., Beijing 100013, China
Fund Project:

摘要: 硫酸盐、铵盐等水溶性无机盐粒子是大气气溶胶的重要组成部分，为进一步提高高效过滤器性能测试实验的精度，提出了过滤器测试标准要求外的新的人工尘气溶胶发生液（NH4）2SO4，并通过一系列实验，从相关性、粒谱分布、分散度等方面对其气溶胶粒子能否满足测试气溶胶的要求进行验证分析。实验结果表明，（NH4）2SO4和KCl间的相关系数R2为0.994 78，相关性很好；NaCl、KCl和（NH4）2SO4气溶胶的几何标准差分别为0.88、0.85和0.87，呈单分散且分散程度接近，可很好的满足测试气溶胶要求。还获得了可控参数喷气压力与发生溶液质量浓度对（NH4）2SO4气溶胶粒谱分布的影响规律：随喷气压力的增加，气溶胶粒子的粒径减小，分布集中；而随发生溶液质量浓度的增加，粒径增大，导致分散度增加。质量浓度和喷气压力对（NH4）2SO4和KCl气溶胶粒径和分散度作用规律的一致性进一步表明（NH4）2SO4作为测试气溶胶的可行性。
- 人工尘气溶胶 /
- 粒谱分布 /
- 相关性 /
- 几何标准差
Abstract: Water-soluble inorganic salt particles, such as sulfate and ammonium salts, are important components of atmospheric aerosol. To improve the accuracy of high-efficiency filter performance tests, a new dust aerosol-generating solution, (NH4)2SO4, is proposed. This solution is different from the test aerosols used in the filter test standards. To verify its ability to meet the requirements of test aerosols, a series of experiments was conducted to evaluate the correlation, particle distribution, and dispersion. The experimental results show that the correlation coefficient R2 between (NH4)2SO4 and KCl is 0.994 78, indicating good correlation. The geometric standard deviations of NaCl, KCl, and (NH4)2SO4 are 0.87, 0.85, and 0.88, respectively, which are all correspond to single dispersion. The variation trend of the new dust aerosol (NH4)2SO4 is consistent with the standard aerosol and can readily satisfy the requirements of test aerosols. In addition, the influence of the jet pressure and solution concentration, as controllable parameters, on the particle size distribution of aerosol (NH4)2SO4 is also determined. With increasing jet pressure, the particle size decreases, and the size distribution becomes more uniform. Meanwhile, with as the solution concentration increases, the particle size and dispersion degree increase. The consistency of the influence of the solution concentration and injection pressure on the particle size and dispersion degree between (NH4)2SO4 and KCl shows that (NH4)2SO4 is a feasible test aerosol.
- artificial dust aerosol /
- particle size distribution /
- correlation /
- geometric standard deviation

[1]	肖沅芷, 沈恒根, 刘兴成. 家居环境PM_2.5控制用空气滤料[J]. 环境工程学报, 2015, 9(5):2347-2352
[2]	中华人民共和国国家质量监督检验检疫总局, 中国国家标准化管理委员会. GB/T 14295-2008空气过滤器[S]. 北京:中国标准出版社, 2009
[3]	住房和城乡建设部. GB/T 6165-2008高效空气过滤器性能实验方法效率和阻力[S]. 北京:中国标准出版社, 2009
[4]	王淑兰, 柴发合, 张远航, 等. 成都市大气颗粒物污染特征及其来源分析[J]. 地理科学, 2004, 24(4):488-492
[5]	张承中, 丁超, 周变红, 等. 西安市冬、夏两季PM_2.5中碳气溶胶的污染特征分析[J]. 环境工程学报, 2013, 7(4):1477-1481
[6]	徐宏辉, 王跃思, 温天雪, 等. 北京大气气溶胶中水溶性离子的粒径分布和垂直分布[J]. 环境科学, 2007, 28(1):14-19
[7]	董雪玲, 刘大锰, 袁杨森, 等. 北京市2005年夏季大气颗粒物污染特征及影响因素[J]. 环境工程学报, 2007, 1(9):100-104
[8]	胡荣章, 刘红年, 张美根, 等. 南京地区大气灰霾的数值模拟[J]. 环境科学学报, 2009, 29(4):808-814
[9]	JANSEN R C, SHI Yang, CHEN Jianmin, et al. Using hourly measurements to explore the role of secondary inorganic aerosol in PM_2.5 during haze and fog in Hangzhou, China[J]. Advances in Atmospheric Sciences, 2014, 31(6):1427-1434
[10]	成天涛, 吕达仁, 陈洪滨, 等. 浑善达克沙地沙尘气溶胶的粒谱特征[J]. 大气科学, 2005, 29(1):147-153
[11]	EPSTEIN B. The mathematical description of certain breakage mechanisms leading to the logarithmico-normal distribution[J]. Journal of Franklin Institute, 1947, 244(6):471-477
[12]	PATTERSON E M, GILLETTE D A. Commonalities in measured size distributions for aerosols having a soil-derived component[J]. Journal of Geophysical Research, 1977, 82(15):2074-2082
[13]	王智超, 宋灿华, 刘志军. Laskin喷嘴喷雾性能实验研究[J]. 暖通空调, 2010, 40(2):133-137

点击查看大图

计量

文章访问数: 2283
HTML全文浏览数: 1786
PDF下载数: 435
施引文献: 0

邓高峰, 李增和, 胡露露, 王智超, 郜津慧. 硫酸铵作为人工气溶胶模拟尘源的研究[J]. 环境工程学报, 2017, 11(2): 977-982. doi: 10.12030/j.cjee.201509193

引用本文:

邓高峰, 李增和, 胡露露, 王智超, 郜津慧. 硫酸铵作为人工气溶胶模拟尘源的研究[J]. 环境工程学报, 2017, 11(2): 977-982. doi: 10.12030/j.cjee.201509193

Citation:

硫酸铵作为人工气溶胶模拟尘源的研究

1. 北京化工大学理学院, 北京 100029
2. 中国建筑科学研究院建筑环境与安全国家重点实验室, 北京 100013
3. 建研科技股份有限公司, 北京 100013

收稿日期: 2015-11-03

基金项目:

国家科技支撑计划项目（2013BAK12B03）

关键词:

摘要: 硫酸盐、铵盐等水溶性无机盐粒子是大气气溶胶的重要组成部分，为进一步提高高效过滤器性能测试实验的精度，提出了过滤器测试标准要求外的新的人工尘气溶胶发生液（NH4）2SO4，并通过一系列实验，从相关性、粒谱分布、分散度等方面对其气溶胶粒子能否满足测试气溶胶的要求进行验证分析。实验结果表明，（NH4）2SO4和KCl间的相关系数R2为0.994 78，相关性很好；NaCl、KCl和（NH4）2SO4气溶胶的几何标准差分别为0.88、0.85和0.87，呈单分散且分散程度接近，可很好的满足测试气溶胶要求。还获得了可控参数喷气压力与发生溶液质量浓度对（NH4）2SO4气溶胶粒谱分布的影响规律：随喷气压力的增加，气溶胶粒子的粒径减小，分布集中；而随发生溶液质量浓度的增加，粒径增大，导致分散度增加。质量浓度和喷气压力对（NH4）2SO4和KCl气溶胶粒径和分散度作用规律的一致性进一步表明（NH4）2SO4作为测试气溶胶的可行性。

English Abstract

Research on ammonium sulfate as artificial aerosol simulated dust source

1. College of Science, Beijing University of Chemical Technology, Beijing 100029, China
2. State Key Laboratory of Building Safety and Built Environment, China Academy of Building Research, Beijing 100013, China
3. Cabr Technology Co. Ltd., Beijing 100013, China

Received Date: 2015-11-03

Fund Project:

Keywords:

Abstract: Water-soluble inorganic salt particles, such as sulfate and ammonium salts, are important components of atmospheric aerosol. To improve the accuracy of high-efficiency filter performance tests, a new dust aerosol-generating solution, (NH4)2SO4, is proposed. This solution is different from the test aerosols used in the filter test standards. To verify its ability to meet the requirements of test aerosols, a series of experiments was conducted to evaluate the correlation, particle distribution, and dispersion. The experimental results show that the correlation coefficient R2 between (NH4)2SO4 and KCl is 0.994 78, indicating good correlation. The geometric standard deviations of NaCl, KCl, and (NH4)2SO4 are 0.87, 0.85, and 0.88, respectively, which are all correspond to single dispersion. The variation trend of the new dust aerosol (NH4)2SO4 is consistent with the standard aerosol and can readily satisfy the requirements of test aerosols. In addition, the influence of the jet pressure and solution concentration, as controllable parameters, on the particle size distribution of aerosol (NH4)2SO4 is also determined. With increasing jet pressure, the particle size decreases, and the size distribution becomes more uniform. Meanwhile, with as the solution concentration increases, the particle size and dispersion degree increase. The consistency of the influence of the solution concentration and injection pressure on the particle size and dispersion degree between (NH4)2SO4 and KCl shows that (NH4)2SO4 is a feasible test aerosol.

全文HTML

参考文献 (13)

下载: 全尺寸图片幻灯片

返回文章

用微信扫码二维码

分享至好友和朋友圈

硫酸铵作为人工气溶胶模拟尘源的研究

Research on ammonium sulfate as artificial aerosol simulated dust source

计量

出版历程

硫酸铵作为人工气溶胶模拟尘源的研究

English Abstract

Research on ammonium sulfate as artificial aerosol simulated dust source

全文HTML

目录